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|a (TOE)ost1348872
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|a E 1.99:1348872
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|a E 1.99:1348872
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|a X-ray absorption spectroscopy using a self-seeded soft X-ray free-electron laser
|h [electronic resource]
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|a Washington, D.C. :
|b United States. Department of Energy. Office of Basic Energy Sciences ;
|a Oak Ridge, Tenn. :
|b distributed by the Office of Scientific and Technical Information, U.S. Department of Energy,
|c 2016.
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|a Article No. 22469 :
|b digital, PDF file.
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|a text
|b txt
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|a computer
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|a online resource
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|a Published through SciTech Connect.
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|a 09/19/2016.
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|a Optics Express 24 20 ISSN 1094-4087; OPEXFF AM.
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|a Thomas Kroll; Jan Kern; Markus Kubin; Daniel Ratner; Sheraz Gul; Franklin D. Fuller; Heike Löchel; Jacek Krzywinski; Alberto Lutman; Yuantao Ding; Georgi L. Dakovski; Stefan Moeller; Joshua J. Turner; Roberto Alonso-Mori; Dennis L. Nordlund; Jens Rehanek; Christian Weniger; Alexander Firsov; Maria Brzhezinskaya; Ruchira Chatterjee; Benedikt Lassalle-Kaiser; Raymond G. Sierra; Hartawan Laksmono; Ethan Hill; Andrew Borovik; et al.
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|a X-ray free electron lasers (XFELs) enable unprecedented new ways to study the electronic structure and dynamics of transition metal systems. L-edge absorption spectroscopy is a powerful technique for such studies and the feasibility of this method at XFELs for solutions and solids has been demonstrated. But, the required x-ray bandwidth is an order of magnitude narrower than that of self-amplified spontaneous emission (SASE), and additional monochromatization is needed. We compare L-edge x-ray absorption spectroscopy (XAS) of a prototypical transition metal system based on monochromatizing the SASE radiation of the linac coherent light source (LCLS) with a new technique based on self-seeding of LCLS. We demonstrate how L-edge XAS can be performed using the self-seeding scheme without the need of an additional beam line monochromator. Lastly, we show how the spectral shape and pulse energy depend on the undulator setup and how this affects the x-ray spectroscopy measurements.
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|b AC02-05CH11231.
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|b AC02-76SF00515.
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|a Instrumentation Related To Nuclear Science And Technology.
|2 edbsc.
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|a SLAC National Accelerator Laboratory.
|4 res.
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|a United States.
|b Department of Energy.
|b Office of Basic Energy Sciences.
|4 spn.
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|a United States.
|b Department of Energy.
|b Office of Scientific and Technical Information.
|4 dst.
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|u http://www.osti.gov/scitech/biblio/1348872
|z Online Access (via OSTI)
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|a .b91181598
|b 03-09-23
|c 05-12-17
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|a web
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|p Can circulate
|a University of Colorado Boulder
|b Online
|c Online
|d Online
|e E 1.99:1348872
|h Superintendent of Documents classification
|i web
|n 1
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